In the coming decade, artificial intelligence systems are set to revolutionise every industry and facet of human life. Building communication systems that enable seamless and symbiotic communication between humans and AI agents is increasingly important. This research advances the field of human-AI interaction by developing an innovative approach to decode imagined speech using non-invasive high-density functional near-infrared spectroscopy (fNIRS). Notably, this study introduces MindGPT, the first thought-to-LLM (large language model) system in the world.