In the context of globalization and the rapid expansion of the digital economy, anti-money laundering (AML) has become a crucial aspect of financial oversight, particularly in cross-border transactions. The rising complexity and scale of international financial flows necessitate more intelligent and adaptive AML systems to combat increasingly sophisticated money laundering techniques. This paper explores the application of unsupervised learning models in cross-border AML systems, focusing on rule optimization through contrastive learning techniques. Five deep learning models, ranging from basic convolutional neural networks (CNNs) to hybrid CNNGRU architectures, were designed and tested to assess their performance in detecting abnormal transactions. The results demonstrate that as model complexity increases, so does the system's detection accuracy and responsiveness. In particular, the self-developed hybrid Convolutional-Recurrent Neural Integration Model (CRNIM) model showed superior performance in terms of accuracy and area under the receiver operating characteristic curve (AUROC). These findings highlight the potential of unsupervised learning models to significantly improve the intelligence, flexibility, and real-time capabilities of AML systems. By optimizing detection rules and enhancing adaptability to emerging money laundering schemes, this research provides both theoretical and practical contributions to the advancement of AML technologies, which are essential for safeguarding the global financial system against illicit activities.