In this paper, the problem of dynamical deployment of unmanned aerial vehicles (UAVs) equipped with visible light communication (VLC) capabilities for optimizing the energy efficiency of UAV-enabled networks is studied. In the studied model, the UAVs can simultaneously provide communications and illumination to service ground users. Since ambient illumination increases the interference over VLC links while reducing the illumination threshold of the UAVs, it is necessary to consider the illumination distribution of the target area for UAV deployment optimization. This problem is formulated as an optimization problem which jointly optimizes UAV deployment, user association, and power efficiency while meeting the illumination and communication requirements of users. To solve this problem, an algorithm that combines the machine learning framework of gated recurrent units (GRUs) with convolutional neural networks (CNNs) is proposed. Using GRUs and CNNs, the UAVs can model the long-term historical illumination distribution and predict the future illumination distribution. Given the prediction of illumination distribution, the original nonconvex optimization problem can be divided into two sub-problems and is then solved using a low-complexity, iterative algorithm. Then, the proposed algorithm enables UAVs to determine the their deployment and user association to minimize the total transmit power. Simulation results using real data from the Earth observations group (EOG) at NOAA/NCEI show that the proposed approach can achieve up to 68.9% reduction in total transmit power compared to a conventional optimal UAV deployment that does not consider the illumination distribution and user association.