Self-normalized processes arise naturally in many learning-related tasks. While self-normalized concentration has been extensively studied for scalar-valued processes, there are few results for multidimensional processes outside of the sub-Gaussian setting. In this work, we construct a general, self-normalized inequality for multivariate processes that satisfy a simple yet broad sub-$ψ$ tail condition, which generalizes assumptions based on cumulant generating functions. From this general inequality, we derive an upper law of the iterated logarithm for sub-$ψ$ vector-valued processes, which is tight up to small constants. We show how our inequality can be leveraged to derive a variety of novel, self-normalized concentration inequalities under both light and heavy-tailed observations. Further, we provide applications in prototypical statistical tasks, such as parameter estimation in online linear regression, autoregressive modeling, and bounded mean estimation via a new (multivariate) empirical Bernstein concentration inequality.