For a graph $Γ=(V(Γ),E(Γ))$, a subset $C$ of $V(Γ)$ is called an $(α,β)$-regular set in $Γ$, if every vertex of $C$ is adjacent to exactly $α$ vertices of $C$ and every vertex of $V(Γ)\setminus C$ is adjacent to exactly $β$ vertices of $C$. In particular, if $C$ is an $(α,β)$-regular set in some Cayley sum graph of a finite group $G$ with connection set $S$, then $C$ is called an $(α,β)$-regular set of $G$. In this paper, we consider a generalized dicyclic group $G$ and for each subgroup $H$ of $G$, by giving an appropriate connection set $S$, we determine each possibility for $(α,β)$ such that $H$ is an $(α,β)$-regular set of $G$.