Let $λ_{2}(G)$ be the second smallest normalized Laplacian eigenvalue of a graph $G$. In this paper, we determine all unicyclic graphs of order $n\geq21$ with $λ_{2}(G)\geq 1-\frac{\sqrt{6}}{3}$. Moreover, the unicyclic graphs with $λ_{2}(G)=1-\frac{\sqrt{6}}{3}$ are also determined.
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