This study investigates the use of large language models (LLMs) for human behavior understanding by jointly leveraging motion and video data. We argue that integrating these complementary modalities is essential for capturing both fine-grained motion dynamics and contextual semantics of human actions, addressing the limitations of prior motion-only or video-only approaches. To this end, we propose ViMoNet, a multimodal vision-language framework trained through a two-stage alignment and instruction-tuning strategy that combines precise motion-text supervision with large-scale video-text data. We further introduce VIMOS, a multimodal dataset comprising human motion sequences, videos, and instruction-level annotations, along with ViMoNet-Bench, a standardized benchmark for evaluating behavior-centric reasoning. Experimental results demonstrate that ViMoNet consistently outperforms existing methods across caption generation, motion understanding, and human behavior interpretation tasks. The proposed framework shows significant potential in assistive healthcare applications, such as elderly monitoring, fall detection, and early identification of health risks in aging populations. This work contributes to the United Nations Sustainable Development Goal 3 (SDG 3: Good Health and Well-being) by enabling accessible AI-driven tools that promote universal health coverage, reduce preventable health issues, and enhance overall well-being.